The current version of Reko is quite crude and could use assistance.
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Support for more processor architectures and platforms. Currently Reko has support for x86, Motorola 68k, and MS-DOS, Win32, ELF, and Hunk executable formats. See the "How to..." wiki page for how to contribute new architectures and platforms.
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GUI: the work on a useful GUI hasn't left the planning stages; ideas about mouse/keyboard interaction to afford a convenient user interface are still mulled.
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Porting to other environments: a Mono/GTK# port is in the works.